T. Paul Bui

In‐situ observations of mid‐latitude forest fire plumes deep in the stratosphere

We observed a plume of air highly enriched in carbon monoxide and particles in the stratosphere at altitudes up to 15.8 km. It can be unambiguously attributed to North American forest fires. This plume demonstrates an extratropical direct transport path from the planetary boundary layer several kilometers deep into the stratosphere, which is not fully captured by large-scale atmospheric transport models. This process indicates that the stratospheric ozone layer could be sensitive to changes in forest burning associated with climatic warming.

Ice nucleation and dehydration in the Tropical Tropopause Layer

Optically thin cirrus near the tropical tropopause regulate the humidity of air entering the stratosphere, which in turn has a strong influence on the Earth’s radiation budget and climate. Recent high-altitude, unmanned aircraft measurements provide evidence for two distinct classes of cirrus formed in the tropical tropopause region: (i) vertically extensive cirrus with low ice number concentrations, low extinctions, and large supersaturations (up to ∼70%) with respect to ice; and (ii) vertically thin cirrus layers with much higher ice concentrations that effectively deplete the vapor in excess of saturation. The persistent supersaturation in the former class of cirrus is consistent with the long time-scales (several hours or longer) for quenching of vapor in excess of saturation given the low ice concentrations and cold tropical tropopause temperatures. The low-concentration clouds are likely formed on a background population of insoluble particles with concentrations less than 100 L−1 (often less than 20 L−1), whereas the high ice concentration layers (with concentrations up to 10,000 L−1) can only be produced by homogeneous freezing of an abundant population of aqueous aerosols. These measurements, along with past high-altitude aircraft measurements, indicate that the low-concentration cirrus occur frequently in the tropical tropopause region, whereas the high-concentration cirrus occur infrequently. The predominance of the low-concentration clouds means cirrus near the tropical tropopause may typically allow entry of air into the stratosphere with as much as ∼1.7 times the ice saturation mixing ratio.

Ice Microphysics Observations in Hurricane Humberto: Comparison with Non-Hurricane-Generated Ice Cloud Layers

Abstract Measurements are presented that were acquired from the National Aeronautics and Space Administration (NASA) DC-8 aircraft during an intensive 3-day study of Tropical Storm/Hurricane Humberto on 22, 23, and 24 September 2001. Particle size distributions, particle image information, vertical velocities, and single- and dual-wavelength Doppler radar observations were obtained during repeated sampling of the eyewall and outer eye regions. Eyewall sampling temperatures ranged from −22° to −57°C and peak updraft velocities from 4 to 15 m s−1. High concentrations of small ice particles, in the order 50 cm−3 and above, were observed within and around the updrafts. Aggregates, some larger than 7 mm, dominated the larger sizes. The slope of the fitted exponential size distributions λ was distinctly different close to the eye than outside of that region. Even at low temperatures, λ was characteristic of warm temperature growth (λ < 30 cm−1) close to the eye and characteristic of low temperature growth outsi...

Ubiquitous influence of waves on tropical high cirrus clouds

Cirrus clouds in the tropical tropopause layer (TTL) and water vapor transported into the stratosphere have significant impacts on the global radiation budget and circulation patterns. Climate models, however, have large uncertainties in representing dehydration and cloud processes in the TTL, and thus their feedback on surface climate, prohibiting an accurate projection of future global and regional climate changes. Here we use unprecedented airborne measurements over the Pacific to reveal atmospheric waves as a strong modulator of ice clouds in the TTL. Wave-induced cold and/or cooling conditions are shown to exert a nearly ubiquitous influence on cirrus cloud occurrence at altitudes of 14–18 km, except when air was very recently influenced by convective hydration. We further observe that various vertical scales of cloud layers are associated with various vertical scales of waves, suggesting the importance of representing TTL waves in models.

A New Instrumented Airborne Platform for Atmospheric Research

AbstractThe NASA Ames Research Center operates a new research platform for atmospheric studies: an instrumented Alpha Jet. The present complement of instruments allows for the determination of carbon dioxide, ozone, water vapor, and methane concentrations as well as measurements of three-dimensional wind speeds, temperature, and pressure. Planned future instrumentation includes an Air-Core sampler and an instrument to measure formaldehyde. We give examples of measurements that have been made, including measurements carried out during a downward spiral over an expected methane source. An attractive property of this airborne system is its ability to respond rapidly to unexpected atmospheric events such as large forest fires or severe air quality events.

A case study of convectively sourced water vapor observed in the overworld stratosphere over the United States

On August 27, 2013, during the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) field mission, NASAs ER-2 research aircraft encountered a region of enhanced water vapor, extending over a depth of approximately 2 km and a minimum areal extent of 20,000 km2 in the stratosphere (375 K to 415 K potential temperature), south of the Great Lakes (42°N, 90°W). Water vapor mixing ratios in this plume, measured by the Harvard Water Vapor instrument, constitute the highest values recorded in situ at these potential temperatures and latitudes. An analysis of geostationary satellite imagery in combination with trajectory calculations links this water vapor enhancement to its source, a deep tropopause-penetrating convective storm system that developed over Minnesota 20 hours prior to the aircraft plume encounter. High resolution, ground-based radar data reveal that this system was comprised of multiple individual storms, each with convective turrets that extended to a maximum of ~4 km above the tropopause level for several hours. In situ water vapor data show that this storm system irreversibly delivered between 6.6 kt and 13.5 kt of water to the stratosphere. This constitutes a 20 – 25% increase in water vapor abundance in a column extending from 115 hP to 70 hPa over the plume area. Both in situ and satellite climatologies show a high frequency of localized water vapor enhancements over the central U.S. in summer, suggesting that deep convection can contribute to the stratospheric water budget over this region and season.