Timothy L. Weiland

Harmonic conversion of large-aperture 1.05-μm laser beams forinertial-confinement fusion research

To provide high-energy, high-power beams at short wavelengths for inertial-confinement fusion experiments, we routinely convert the 1.05-microm output of the Nova, Nd:phosphate-glass, laser system to its second- or third-harmonic wavelength. We describe the design and performance of the 3 x 3 arrays of potassium dihydrogen phosphate crystal plates used for type-II-type-II phase-matched harmonic conversion of the Nova 0.74-m diameter beams. We also describe an alternate type-I-type-II phasematching configuration that improves third-harmonic conversion efficiency. These arrays provide conversion of a Nova beam of up to 75% to the second harmonic and of up to 70% to the third harmonic.

Noncritically phase-matched fourth harmonic generation of Nd:glass lasers in partially deuterated KDP crystals.

Noncritically phase-matched (NCPM) fourth harmonic generation (FHG) of Nd:glass laser radiation in partially deuterated dihydrogen phosphate (KD*P) crystals has been demonstrated. At an Nd:glass laser wavelength of 1053.0 nm, NCPM FHG is achieved in 70% deuterated KD*P at a crystal temperature of 18.5±0.1 °C. Tuning the fundamental laser wavelength from 1052.9 to 1053.2 nm, FHG in KD*P is NCPM by changing the crystal temperature from 17.9 °C to 20.5 °C. When driven with 2.4 J of second harmonic radiation in a 3 ns flat-top pulse, corresponding to 1 GW/cm(2) 2ω drive intensity, 1.9 J of fourth harmonic radiation was generated in a 6 mm long KD*P crystal, yielding a second to fourth harmonic energy conversion efficiency of 79%.

Pulse length dependence of laser conditioning and bulk damage in KD2PO4

An experimental technique has been developed to measure the damage density ρ(Φ) variation with fluence from scatter maps of bulk damage sites in plates of KD2PO4 (DKDP) crystals combined with calibrated images of the damaging beams spatial profile. Unconditioned bulk damage in tripler-cut DKDP crystals has been studied using 351 nm (3ω) light at pulse lengths of 0.055, 0.091, 0.30, 0.86, 2.6, and 10 ns. It is found that there is less scatter due to damage at fixed fluence for longer pulse lengths. The results also show that for all the pulse lengths the scatter due to damage is a strong function of the damaging fluence. It is determined that the pulse length scaling for bulk damage scatter in unconditioned DKDP material varies as τ0.24±0.05 over two orders of magnitude of pulse lengths. The effectiveness of 3ω laser conditioning at pulse lengths of 0.055, 0.096, 0.30, 0.86, 3.5, and 23 ns is analyzed in term of damage density ρ(Φ) at 3ω, 2.6 ns. The 860 ps conditioning to a peak irradiance of 7 GW/cm2 had the best performance under 3ω, 2.6 ns testing. It is shown that the optimal conditioning pulse length appears to lies in the range from 0.3 to 1 ns with a low sensitivity of 0.5 J/cm2/ns to the exact pulse length.

Laser damage performance of fused silica optical components measured on the beamlet laser at 351 nm

A statistics-based model is being developed to predict the laser-damage-limited lifetime of UV optical components on the NIF laser. in order to provide data for the model, laser damage experiments were performed on the Beamlet laser system at LLNL. Three prototype NIF focus lenses were exposed to 351 nm pulses during four experimental campaigns, each consisting of 23 to 38 pulses at NIF relevant fluences. Each lens was sol-gel AR coated and all laser exposures were performed in a vacuum environment. Through inspections of the lens before, during and after the campaigns, pulse-to- pulse damage growth rates were measured for damage initiating both on the surfaces and at bulk inclusions. Radial growth rates measured for rear surface damage was typically 10x higher than that measured in the bulk or at the front surface. No significant correlation of growth rate to precursor type was indicated. For 5 J/cm2, 3 ns pulses the typical radial growth rate was nominally 20 micrometers /pulse. Average growth rates measured on three lenses made by two manufacturers were in good agreement. While the growth rate clearly increased with fluence, the data obtained was insufficient to quantify the dependence. The growth rates reported here were 20x-50x higher than values predicted from off-line studies of bare surfaces in air.

Power, energy, and temporal performance of the Nova laser facility with recent improvements to the amplifier system

High-powered glass-laser systems with multiple beams, frequency-conversion capabilities, and pulseshaping flexibility have made numerous contributions to the understanding of inertial confinement fusion and related laser-plasma interactions. The Nova laser at Lawrence Livermore National Laboratory is the largest such laser facility. We have made improvements to the Nova amplifier system that permit increased power and energy output. We summarize the nonlinear effects that now limit Novas performance and discuss power and energy produced at 1.05-, 0.53-, and 0.35-microm wavelengths, including the results with pulses temporally shaped to improve inertial confinement fusion target performance.

Wavelength and pulselength dependence of laser conditioning and bulk damage in doubler-cut KH2PO4

An experimental technique has been utilized to measure the variation of bulk damage scatter with damaging fluence in plates of KH2PO4 (KDP) crystals. Bulk damage in unconditioned and laser-conditioned doubler-cut KDP crystals has been studied using 527 nm (2ω) light at pulselengths of 0.3 - 10 ns. It is found that there is less scatter due to damage at fixed fluence for longer pulselengths. In particular, there is ~4X increase in fluence for equivalent scatter for damage at 2ω, 10 ns as compared to 0.30 ns in unconditioned KDP. The results for the unconditioned and conditioned KDP show that for all the pulselengths the scatter due to the bulk damage is a strong function of the damaging fluence (θ~5). It is determined that the 2ω fluence pulselength-scaling for equivalent bulk damage scatter in unconditioned KDP varies as τ0.30±0.11 and in 3ω, 3ns ramp-conditioned KDP varies as τ0.27±0.14. The effectiveness of 2ω and 3ω laser conditioning at pulselengths in the range of 0.30-23 ns for damage induced 2ω, 3 ns is analyzed in terms of scatter. For the protocols tested (i.e. peak conditioning irradiance, etc.), the 3ω, 300 ps conditioning to a peak fluence of 3 J/cm2 had the best performance under 2ω, 3 ns testing. The general trend in the performance of the conditioning protocols was shorter wavelength and shorter pulselength appear to produce better conditioning for testing at 2ω, 3 ns.

Engineering meter-scale laser resistant coatings for the near IR

Laser resistant coatings are needed for beam steering (mirrors), pulse switching (polarizers), and high transport efficiency on environmental barriers (windows / lenses) on large laser systems. A range of defects limit the exposure fluence of these coatings. By understanding the origin and damage mechanisms for these defects, the deposition process can be optimized to realize coatings with greater laser resistance. Electric field modeling can provide insight into which defects are most problematic. Laser damage growth studies are useful for determining a functional laser damage criteria. Mitigation techniques such as micro-machining with a single-crystal diamond cutting tool or short pulse laser ablation using the burst technique can be used to arrest growth in damage sites to extend optic lifetime.

Temporal shaping of third-harmonic pulses on the Nova laser system

We demonstrate temporal shaping of 0.35-microm-wavelength pulses produced by a third-harmonic conversion of the output from the Nova Nd:phosphate glass-laser amplifier system for use in inertial confinement fusion experiments. We describe the computer models used to calculate the pulse shape that is required as the input to the amplifier system, the experimental apparatus used to produce these pulses, and the high-power 0.35-microm shaped pulses produced in recent experiments.

Wavefront and divergence of the beamlet prototype laser

We have measured the wavefront and the divergence of the Beamlet prototype laser under a variety of conditions. Emphasis of the tests was on quantifying best attainable divergence in the angular regime below 30 (mu) rad to benchmark propagation models that are used to set wavefront gradient specifications for NIF optical components. Performance with and without active wavefront correction was monitored with radial shearing interferometers that measured near-field wavefront at the input and output of the main amplifier with a spatial resolution of 1 cm, and cameras which measured the corresponding intensity distributions in the far field with an angular resolution of 0.3 (Mu) rad. Details of the measurements are discussed and related to NIF focal spot requirements and optics specifications.

Effect of bandwidth on beam smoothing and frequency conversion at the third harmonic of the Nova laser

We present the results of experiments performed on the Nova laser system to determine the effect of bandwidth on third harmonic (3(omega) ) frequency conversion and beam smoothing by spectral dispersion (SSD). Our experiments utilized a wide bandwidth fiber optic cross- phase modulated (XPM) source and a narrower bandwidth microwave modulated (FM) source, each centered at 1053 nm (1 (omega) ). A significant fraction (> 50%) of the 1(omega) XPM bandwidth was transferred to the 3(omega) beam (22 cm-1 yields 36 cm-1), yielding 0.13% bandwidth at 3(omega) . The maximum intrinsic narrowband 3(omega) frequency conversion obtained using a type-II/type-II KDP crystal array was 62%. The intrinsic efficiency obtained at the Nova 10-beam chamber is typically > 65%. Frequency conversion was essentially unaffected by the 2 cm-1 bandwidth obtained from FM source. However, the 5 - 16 cm-1 of bandwidth from the XPM source reduced the conversion efficiency to approximately 24%. We have developed broadband frequency conversion codes and broadband pulse simulations to model our results, and have obtained good agreement with experiment.