Mark C. Rosamond

Surface acoustic wave generation and detection using graphene interdigitated transducers on lithium niobate

We demonstrate the feasibility of using graphene as a conductive electrode for the generation and detection of surface acoustic waves at 100 s of MHz on a lithium niobate substrate. The graphene interdigitated transducers (IDTs) show sensitivity to doping and temperature, and the characteristics of the IDTs are discussed in the context of a lossy transmission line model.

Excitation, detection, and electrostatic manipulation of terahertz-frequency range plasmons in a two-dimensional electron system.

Terahertz frequency time-domain spectroscopy employing free-space radiation has frequently been used to probe the elementary excitations of low-dimensional systems. The diffraction limit, however, prevents its use for the in-plane study of individual laterally-defined nanostructures. Here, we demonstrate a planar terahertz frequency plasmonic circuit in which photoconductive material is monolithically integrated with a two-dimensional electron system. Plasmons with a broad spectral range (up to ~ 400 GHz) are excited by injecting picosecond-duration pulses, generated and detected by a photoconductive semiconductor, into a high mobility two-dimensional electron system. Using voltage modulation of a Schottky gate overlying the two-dimensional electron system, we form a tuneable plasmonic cavity, and observe electrostatic manipulation of the plasmon resonances. Our technique offers a direct route to access the picosecond dynamics of confined electron transport in a broad range of lateral nanostructures.

Spin relaxation through Kondo scattering in Cu/Py lateral spin valves.

The temperature dependence of the spin diffusion length typically reflects the scattering mechanism responsible for spin relaxation. Within non-magnetic metals it is reasonable to expect the Elliot-Yafet mechanism to play a role and thus the temperature dependence of the spin diffusion length might be inversely proportional to resistivity. In lateral spin valves measurements have found that at low temperatures the spin diffusion length unexpected decreases. By measuring the transport properties of lateral Py/Cu/Py spin valves fabricated with different purities of Cu, we extract a spin diffusion length which shows this suppression below 30K only in the presence of the Kondo effect. We have calculated the spin-relaxation rate and isolated the contributions from magnetic impurities. We find the spin-flip probability of a magnetic impurity to be 34%. Our semi-quantitative analysis demonstrates the dominant role of Kondo scattering in spin relaxation, even in low concentrations of order 1 p.p.m., and hence accounts for the reduction in spin diffusion length observed by ourselves and others.

Brillouin light scattering study of magnetic-element normal modes in a square artificial spin ice geometry

We report the results, from experimental and micromagnetic studies, of the magnetic normal modes in artificial square spin ice systems consisting of ferromagnetic-monodomain islands. Spin-wave properties are measured by Brillouin light scattering. The mode spectra contain several branches whose frequencies are sensitive to the magnitude and in-plane orientation of an applied magnetic field. We also identify soft modes that exhibit different behaviours depending on the direction of the applied magnetic field. The obtained results are well described with micromagnetic simulations of independent magnetic elements arranged along two sublattices.

Generation of continuous wave terahertz frequency radiation from metal-organic chemical vapour deposition grown Fe-doped InGaAs and InGaAsP

We demonstrate the generation of continuous wave terahertz (THz) frequency radiation from photomixers fabricated on both Fe-doped InGaAs and Fe-doped InGaAsP, grown by metal-organic chemical vapor deposition. The photomixers were excited using a pair of distributed Bragg reflector lasers with emission around 1550 nm, and THz radiation was emitted over a bandwidth of greater than 2.4 THz. Two InGaAs and four InGaAsP wafers with different Fe doping concentrations were investigated, with the InGaAsmaterial found to outperform the InGaAsP in terms of emitted THz power. The dependencies of the emitted power on the photomixer applied bias, incident laser power, and materialdoping level were also studied.

Ballistic rectification of vortex domain wall chirality at nanowire corners

The interactions of vortex domain walls with corners in planar magnetic nanowires are probed using magnetic soft X-ray transmission microscopy. We show that when the domain walls are propagated into sharp corners using applied magnetic fields above a critical value, their chiralities are rectified to either clockwise or anticlockwise circulation depending on whether the corners turn left or right. Single-shot focused magneto-optic Kerr effect measurements are then used to demonstrate how, when combined with modes of domain propagation that conserve vortex chirality, this allows us to dramatically reduce the stochasticity of domain pinning at artificial defect sites. Our results provide a tool for controlling domain wall chirality and pinning behavior both in further experimental studies and in future domain wall-based memory, logic and sensor technologies.

Fabrication of a Horizontal and a Vertical Large Surface Area Nanogap Electrochemical Sensor

Nanogap sensors have a wide range of applications as they can provide accurate direct detection of biomolecules through impedimetric or amperometric signals. Signal response from nanogap sensors is dependent on both the electrode spacing and surface area. However, creating large surface area nanogap sensors presents several challenges during fabrication. We show two different approaches to achieve both horizontal and vertical coplanar nanogap geometries. In the first method we use electron-beam lithography (EBL) to pattern an 11 mm long serpentine nanogap (215 nm) between two electrodes. For the second method we use inductively-coupled plasma (ICP) reactive ion etching (RIE) to create a channel in a silicon substrate, optically pattern a buried 1.0 mm × 1.5 mm electrode before anodically bonding a second identical electrode, patterned on glass, directly above. The devices have a wide range of applicability in different sensing techniques with the large area nanogaps presenting advantages over other devices of the same family. As a case study we explore the detection of peptide nucleic acid (PNA)−DNA binding events using dielectric spectroscopy with the horizontal coplanar device.

Thickness dependence of spin wave excitations in an artificial square spin ice-like geometry

We present a comparative study of the spin wave properties in two magnetic films patterned into an artificial square spin ice-like geometry. The array elements are rectangular islands with the same lateral dimensions but with different thicknesses: 10 nm and 30 nm. Using Brillouin light scattering, the frequencies of spin wave excitations were measured as a function of the magnetic field going from positive to negative saturation. We find substantial changes with thickness to spin wave mode frequencies and the number of detected modes. Frequencies of spin waves localized at element edges are observed to evolve non-monotonically with magnetic fields and soften at critical fields. These critical fields enable us to extract information of the magnetization reversal of individual islands within the array. Finally, we discuss the effects of separation between islands and examine the possibilities for dynamic coupling through the overlap of collective edge modes.

Observation of spin-wave Doppler shift in Co90Fe10/Ru micro-strips for evaluating spin polarization

The current-induced spin-wave Doppler shift has been investigated for Co90Fe10 films, with and without under- and overlayers of Ru, aiming to obtain quantitative insights into the value of spin polarization of the diffusive electrical currents flowing in this material. This extends the use of spin-wave Doppler shift spectroscopy beyond the study of permalloy to other soft magnetic materials suitable for use in spintronic applications such as racetrack memories. The Damon-Eshbach spin-wave mode was employed, and a control experiment of permalloy yielded a value of spin polarization of P = 0.44 ± 0.03 for that material. An extended method to properly evaluate spin-wave Doppler shifts is developed that takes account of the non-negligible Oersted fields that are generated by the current density asymmetry caused by conducting under- or overlayers. The values of spin polarization for various Co90Fe10-based structures are found to lie in the range of 0.3–0.35, only slightly less than in permalloy.

Silver-based surface plasmon waveguide for terahertz quantum cascade lasers

Terahertz-frequency quantum cascade lasers (THz QCLs) based on ridge waveguides incorporating silver waveguide layers have been investigated theoretically and experimentally, and compared with traditional gold-based devices. The threshold gain associated with silver-, gold- and copper-based devices, and the effects of titanium adhesion layers and top contact layers, in both surface-plasmon and double-metal waveguide geometries, have been analysed. Our simulations show that silver-based waveguides yield lower losses for THz QCLs across all practical operating temperatures and frequencies. Experimentally, QCLs with silver-based surface-plasmon waveguides were found to exhibit higher operating temperatures and higher output powers compared to those with identical but gold-based waveguides. Specifically, for a three-well resonant phonon active region with a scaled oscillator strength of 0.43 and doping density of 6.83 × 1015 cm-3, an increase of 5 K in the maximum operating temperature and 40% increase in the output power were demonstrated. These effects were found to be dependent on the active region design, and greater improvements were observed for QCLs with a larger radiative diagonality. Our results indicate that silver-based waveguide structures could potentially enable THz QCLs to operate at high temperatures.