Nicolas Bergeard

TEMPO: a New Insertion Device Beamline at SOLEIL for Time Resolved Photoelectron Spectroscopy Experiments on Solids and Interfaces

A new insertion device beamline is now operational on straight section 8 at the SOLEIL synchrotron radiation source in France. The beamline and the experimental station were developed to optimize the study of the dynamics of electronic and magnetic properties of materials. Here we present the main technical characteristics of the installation and the general principles behind them. The source is composed of two APPLE II type insertion devices. The monochromator with plane gratings and spherical mirrors is working in the energy range 40–1500 eV. It is equipped with VLS, VGD gratings to allow the user optimization of flux or higher harmonics rejection. The observed resonance structures measured in gas phase enable us to determine the available energy resolution: a resolving power higher than 10000 is obtained at the Ar 2p, N 1s and Ne K‐edges when using all the optical elements at full aperture. The total flux as a function of the measured photon energy and the characterization of the focal spot size comple...

Time‐resolved photoelectron spectroscopy using synchrotron radiation time structure

Synchrotron radiation time structure is becoming a common tool for studying dynamic properties of materials. The main limitation is often the wide time domain the user would like to access with pump-probe experiments. In order to perform photoelectron spectroscopy experiments over time scales from milliseconds to picoseconds it is mandatory to measure the time at which each measured photoelectron was created. For this reason the usual CCD camera-based two-dimensional detection of electron energy analyzers has been replaced by a new delay-line detector adapted to the time structure of the SOLEIL synchrotron radiation source. The new two-dimensional delay-line detector has a time resolution of 5 ns and was installed on a Scienta SES 2002 electron energy analyzer. The first application has been to characterize the time of flight of the photoemitted electrons as a function of their kinetic energy and the selected pass energy. By repeating the experiment as a function of the available pass energy and of the kinetic energy, a complete characterization of the analyzer behaviour in the time domain has been obtained. Even for kinetic energies as low as 10 eV at 2 eV pass energy, the time spread of the detected electrons is lower than 140 ns. These results and the time structure of the SOLEIL filling modes assure the possibility of performing pump-probe photoelectron spectroscopy experiments with the time resolution given by the SOLEIL pulse width, the best performance of the beamline and of the experimental station.

Ultrafast angular momentum transfer in multisublattice ferrimagnets

Femtosecond laser pulses can be used to induce ultrafast changes of the magnetization in magnetic materials. However, one of the unsolved questions is that of conservation of the total angular momentum during the ultrafast demagnetization. Here we report the ultrafast transfer of angular momentum during the first hundred femtoseconds in ferrimagnetic Co0.8Gd0.2 and Co0.74Tb0.26 films. Using time-resolved X-ray magnetic circular dichroism allowed for time-resolved determination of spin and orbital momenta for each element. We report an ultrafast quenching of the magnetocrystalline anisotropy and show that at early times the demagnetization in ferrimagnetic alloys is driven by the local transfer of angular momenta between the two exchange-coupled sublattices while the total angular momentum stays constant. In Co0.74Tb0.26 we have observed a transfer of the total angular momentum to an external bath, which is delayed by ~150 fs.

Electrical characterization of all-optical helicity-dependent switching in ferromagnetic Hall crosses

We present an experimental study of all-optical helicity-dependent switching (AO-HDS) of ferromagnetic Pt/Co/Pt heterostructures with perpendicular magnetic anisotropy. The sample is patterned into a Hall cross and the AO-HDS is measured via the anomalous Hall effect. This all-electrical probing of the magnetization during AO-HDS enables a statistical quantification of the switching ratio for different laser parameters, such as the threshold power to achieve AO-HDS and the exposure time needed to reach complete switching at a given laser power. We find that the AO-HDS is a cumulative process, a certain number of optical pulses is needed to obtain a full and reproducible helicity-dependent switching. The deterministic switching of the ferromagnetic Pt/Co/Pt Hall cross provides a full “opto-spintronic device,” where the remanent magnetization can be all-optically and reproducibly written and erased without the need of an external magnetic field.

Carbon contamination of soft X-ray beamlines: dramatic anti-reflection coating effects observed in the 1 keV photon energy region.

Carbon contamination is a general problem of under-vacuum optics submitted to high fluence. In soft X-ray beamlines carbon deposit on optics is known to absorb and scatter radiation close to the C K-edge (280 eV), forbidding effective measurements in this spectral region. Here the observation of strong reflectivity losses is reported related to carbon deposition at much higher energies around 1000 eV, where carbon absorptivity is small. It is shown that the observed effect can be modelled as a destructive interference from a homogeneous carbon thin film.

Role of critical spin fluctuations in ultrafast demagnetization of transition-metal rare-earth alloys

Ultrafast magnetization dynamics induced by femtosecond laser pulses have been measured in ferrimagnetic Co0.8Gd0.2, Co0.74Tb0.26, and Co0.86Tb0.14 alloys. Using element sensitivity of x- ray magnetic circular dichroism at the Co L-3, Tb M-5, and Gd M-5 edges, we see that the demagnetization dynamics is element dependent. We show that a thermalization time as fast as 280 +/- 30 fs is observed for the rare earth in the alloy when the excited-state temperature is below the compensation temperature. It is limited to 500 +/- 100 fs when the excited-state temperature is below the Curie temperature (T-C). Therefore, for transition-metal rare-earth alloys, we propose that critical spin fluctuations in the vicinity of T-C reduce the demagnetization rates of the 4f electrons, whereas far from T-C the limited demagnetization rates should be avoided.

Magnetization textures in NiPd nanostructures

nanostructures using three differentimaging techniques: magnetic force microscopy, photoemission electron microscopy under polarizedX-ray absorption, and scanning electron microscopy with polarization analysis. The appearances ofdiamond-like domains with strong lateral charges and of weak stripe structures bring into evidencethe presence of both a transverse and a perpendicular anisotropy in these nanostrips. This anisotropyis seen to reinforce as temperature decreases, as testified by a simplified domain structure at 150 K.A thermal stress relaxation model is proposed to account for these observations. Elastic calculationscoupled to micromagnetic simulations support qualitatively this model.I. INTRODUCTION

Structural dynamics during laser-induced ultrafast demagnetization

Funding from the European Communitys Seventh Framework Programme under Grant Agreement No. 312284 (CALIPSO Project) is gratefully acknowledged, as well as financial support received from the following agencies: (i) The French “Agence National de la Recherche” (ANR) via the projects UMAMI, ANR-11-LABX-0058_NIE and the EQUIPEX UNION (ANR-10-EQPX-52), and (ii) the CNRS-PICS program.

Irreversible transformation of ferromagnetic ordered stripe domains in single-shot infrared-pump/resonant-x-ray-scattering-probe experiments

The evolution of a magnetic domain structure upon excitation by an intense, femtosecond infrared (IR) laser pulse has been investigated using single-shot based time-resolved resonant x-ray scattering at the x-ray free electron laser LCLS. A well-ordered stripe domain pattern as present in a thin CoPd alloy film has been used as a prototype magnetic domain structure for this study. The fluence of the IR laser pump pulse was sufficient to lead to an almost complete quenching of the magnetization within the ultrafast demagnetization process taking place within the first few hundreds of femtoseconds following the IR laser pump pulse excitation. On longer time scales this excitation gave rise to subsequent irreversible transformations of the magnetic domain structure. Under our specific experimental conditions, it took about 2 ns before the magnetization started to recover. After about 5 ns the previously ordered stripe domain structure had evolved into a disordered labyrinth domain structure. Surprisingly, we observe after about 7 ns the occurrence of a partially ordered stripe domain structure reoriented into a novel direction. It is this domain structure in which the samples magnetization stabilizes as revealed by scattering patterns recorded long after the initial pump-probe cycle. Using micromagnetic simulations we can explain this observation based on changes of the magnetic anisotropy going along with heat dissipation in the film.

High-Speed Superconducting Single Photon Detectors for innovative astronomical applications

Superconducting Single Photon Detectors (SSPD) are now mature enough to provide extremely interesting detector performances in term of sensitivity, speed, and geometry in the visible and near infrared wavelengths. Taking advantage of recent results obtained in the Sinphonia project, the goal of our research is to demonstrate the feasibility of a new family of micro-spectrometers, called SWIFTS (Stationary Wave Integrated Fourier Transform Spectrometer), associated to an array of SSPD, the whole assembly being integrated on a monolithic sapphire substrate coupling the detectors array to a waveguide injecting the light. This unique association will create a major breakthrough in the domain of visible and infrared spectroscopy for all applications where the space and weight of the instrument is limited. SWIFTS is an innovative way to achieve very compact spectro-detectors using nano-detectors coupled to evanescent field of dielectric integrated optics. The system is sensitive to the interferogram inside the dielectric waveguide along the propagation path. Astronomical instruments will be the first application of such SSPD spectrometers. In this paper, we describes in details the fabrication process of our SSPD built at CEA/DRFMC using ultra-thin NbN epitaxial films deposited on different orientations of Sapphire substrates having state of the art superconducting characteristics. Electron beam lithography is routinely used for patterning the devices having line widths below 200 nm and down to 70 nm. An experimental set-up has been built and used to test these SSPD devices and evaluate their photon counting performances. Photon counting performances of our devices have been demonstrated with extremely low dark counts giving excellent signal to noise ratios. The extreme compactness of this concept is interesting for space spectroscopic applications. Some new astronomical applications of such concept are proposed in this paper.