Armin Hoffmann

High photon flux table-top coherent extreme-ultraviolet source

High photon flux with up to 1012 photons in the 25–40 eV range has been achieved in a new table-top coherent extreme ultraviolet (EUV) source based on phase-matched high-harmonic generation using a fibre laser. Intense and compact EUV sources are needed for certain types of spectroscopic and imaging applications.

53 W average power few-cycle fiber laser system generating soft x rays up to the water window

We report on a few-cycle laser system delivering sub-8-fs pulses with 353 μJ pulse energy and 25 GW of peak power at up to 150 kHz repetition rate. The corresponding average output power is as high as 53 W, which represents the highest average power obtained from any few-cycle laser architecture so far. The combination of both high average and high peak power provides unique opportunities for applications. We demonstrate high harmonic generation up to the water window and record-high photon flux in the soft x-ray spectral region. This tabletop source of high-photon flux soft x rays will, for example, enable coherent diffractive imaging with sub-10-nm resolution in the near future.

High-repetition-rate and high-photon-flux 70 eV high-harmonic source for coincidence ion imaging of gas-phase molecules

Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced the field by enabling advanced pump-probe schemes. There is an increasing interest in using table-top photon sources enabled by high-harmonic generation of ultrashort-pulse lasers for such studies. We present a novel high-harmonic source driven by a 100 kHz fiber laser system, which delivers 1011 photons/s in a single 1.3 eV bandwidth harmonic at 68.6 eV. The combination of record-high photon flux and high repetition rate paves the way for time-resolved studies of the dissociation dynamics of inner-shell ionized molecules in a coincidence detection scheme. First coincidence measurements on CH3I are shown and it is outlined how the anticipated advancement of fiber laser technology and improved sample delivery will, in the next step, allow pump-probe studies of ultrafast molecular dynamics with table-top XUV-photon sources. These table-top sources can provide significantly higher repetition rates than the currently operating free-electron lasers and they offer very high temporal resolution due to the intrinsically small timing jitter between pump and probe pulses.

Scalability of components for kW-level average power few-cycle lasers.

In this paper, the average power scalability of components that can be used for intense few-cycle lasers based on nonlinear compression of modern femtosecond solid-state lasers is investigated. The key components of such a setup, namely, the gas-filled waveguides, laser windows, chirped mirrors for pulse compression and low dispersion mirrors for beam collimation, focusing, and beam steering are tested under high-average-power operation using a kilowatt cw laser. We demonstrate the long-term stable transmission of kW-level average power through a hollow capillary and a Kagome-type photonic crystal fiber. In addition, we show that sapphire substrates significantly improve the average power capability of metal-coated mirrors. Ultimately, ultrabroadband dielectric mirrors show negligible heating up to 1 kW of average power. In summary, a technology for scaling of few-cycle lasers up to 1 kW of average power and beyond is presented.

Acousto-optic pulse picking scheme with carrier-frequency-to-pulse-repetition-rate synchronization

We introduce and experimentally validate a pulse picking technique based on a travelling-wave-type acousto-optic modulator (AOM) having the AOM carrier frequency synchronized to the repetition rate of the original pulse train. As a consequence, the phase noise characteristic of the original pulse train is largely preserved, rendering this technique suitable for applications requiring carrier-envelope phase stabilization. In a proof-of-principle experiment, the 1030-nm spectral part of an 74-MHz, carrier-envelope phase stable Ti:sapphire oscillator is amplified and reduced in pulse repetition frequency by a factor of two, maintaining an unprecedentedly low carrier-envelope phase noise spectral density of below 68 mrad. Furthermore, a comparative analysis reveals that the pulse-picking-induced additional amplitude noise is minimized, when the AOM is operated under synchronicity. The proposed scheme is particularly suitable when the down-picked repetition rate is still in the multi-MHz-range, where Pockels cells cannot be applied due to piezoelectric ringing.

Concept for CEP-stable few-cycle pulses at 100 W average power

We present the system design and first experimental results of the ELI-ALPS HR1 laser system. At the output CEP-stable few-cycle pulses with 1 mJ energy, >0.1 TW peak power and 100 W of average power will be generated.

High Photon Flux 70 eV HHG Source for Applications in Molecular and Solid State Physics

A 100 kHz high harmonic source with record high >1011 photons/s in single harmonics between 55-73 eV is presented. The unique capabilities are underlined by using it for coincidence experiments and measurements on magnetic samples.

22GW peak power femtosecond fiber CPA system

Over the last decade, the performance of femtosecond fiber laser systems has been rapidly improved. However, further improvements might be held back due to different physical limitations such as nonlinearities or optically induced damage. We demonstrate that with the coherent combination of four parallel fiber amplifiers record pulse energies and peak-powers of 5.7 mJ and 22 GW, respectively, could be achieved. These values could be realized with a chirped-pulse-amplification (CPA) laser system running at a repetition rate of 40 kHz and delivering a compressed average power of 230 W. A high combination efficiency of 89% was achieved demonstrating the scalability of the combining approach to a larger number of channels.

2.1mJ 210W femtosecond fiber CPA system

The coherent combining of ultrashort pulses is a concept for scaling the pulse energy and average power of laser systems emitting ultrashort pulses. This concept has already been demonstrated for two-channel systems. In this contribution we report on a four-channel system that delivers 2.1 mJ pulse energies at a repetition rate of 100 kHz and 210 W of average power after compression. A combination efficiency of 88% was achieved and this demonstrates the scalability of the combining approach to a larger number of channels.

Standoff Sources of Coherent Radiation Initiated by Femtosecond Filaments

we present the results of experimental and theoretical investigations for remote initiation of lasing in nitrogen and air by femtosecond filaments generated by laser pulses with different wavelengths, polarization and applying adaptive control methods